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Which Surface Is More Scaling Resistant? A Closer Look at Nucleation Theories for Heterogeneous Gypsum Nucleation in Aqueous Solutions

https://doi.org/10.1021/acs.est.2c06560

Yin, Yiming ; Li, Tianshu ; Zuo, Kuichang ; Liu, Xitong ; Lin, Shihong ; Yao, Yiqun ; Tong, Tiezheng ( November 2022 , Environmental Science & Technology)

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Wetting, Scaling, and Fouling in Membrane Distillation: State-of-the-Art Insights on Fundamental Mechanisms and Mitigation Strategies

https://doi.org/10.1021/acsestengg.0c00025

Horseman, Thomas ; Yin, Yiming ; Christie, Kofi SS ; Wang, Zhangxin ; Tong, Tiezheng ; Lin, Shihong ( January 2021 , ACS ES&T Engineering)
null (Ed.)
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Distinct Behaviors between Gypsum and Silica Scaling in Membrane Distillation

https://doi.org/10.1021/acs.est.9b06023

Christie, Kofi S. ; Yin, Yiming ; Lin, Shihong ; Tong, Tiezheng ( December 2019 , Environmental Science & Technology)

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Trade-off in membrane distillation with monolithic omniphobic membranes

https://doi.org/10.1038/s41467-019-11209-6

Wang, Wei ; Du, Xuewei ; Vahabi, Hamed ; Zhao, Song ; Yin, Yiming ; Kota, Arun K. ; Tong, Tiezheng ( July 2019 , Nature Communications)

Abstract
Omniphobic membranes are attractive for membrane distillation (MD) because of their superior wetting resistance. However, a design framework for MD membrane remains incomplete, due to the complexity of omniphobic membrane fabrication and the lack of fundamental relationship between wetting resistance and water vapor permeability. Here we present a particle-free approach that enables rapid fabrication of monolithic omniphobic membranes for MD desalination. Our monolithic omniphobic membranes display excellent wetting resistance and water purification performance in MD desalination of hypersaline feedwater containing surfactants. We identify that a trade-off exists between wetting resistance and water vapor permeability of our monolithic MD membranes. Utilizing membranes with tunable wetting resistance and permeability, we elucidate the underlying mechanism of such trade-off. We envision that our fabrication method as well as the mechanistic insight into the wetting resistance-vapor permeability trade-off will pave the way for smart design of MD membranes in diverse water purification applications.

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